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Paper · 2002.07264 · 2020

Combining SchNet and SHARC: The SchNarc machine learning approach for excited-state dynamics

arXiv · PDF · Open in the Atlas

Code that ran

We lifted 8 functions out of this paper's own repositories and ran 5 of them in a sandbox. "Ran" means the function executed on a synthesized input and returned a value. It is not a reproduction of the paper's results.

RepositoryRoleRan
schnarc/schnarc canonical 5 of 8
FunctionStatusWhere it lives
get_diab Ran schnarc/schnarc/src/schnarc/schnarc.py
code served (permissive licence) · get_code("772cc49a755745ff")
get_socs Ran schnarc/schnarc/src/schnarc/schnarc.py
code served (permissive licence) · get_code("a989d6462566487a")
phaseless_loss Ran schnarc/schnarc/src/schnarc/nn.py
code served (permissive licence) · get_code("2a8a3609011f9f81")
read_tradeoffs Ran schnarc/schnarc/src/schnarc/utils.py
code served (permissive licence) · get_code("85d12cfff8578b15")
read_zmat Ran schnarc/schnarc/src/schnarc/utils.py
code served (permissive licence) · get_code("3030ee01ab9feac8")
diagonal_phaseloss Not yet run schnarc/schnarc/src/schnarc/nn.py
code served (permissive licence) · get_code("a969d8293fb86775")
get_schnarc Not yet run schnarc/schnarc/src/schnarc/schnarc.py
code served (permissive licence) · get_code("f1138a9ae711e193")
read_QMout Not yet run schnarc/schnarc/src/schnarc/utils.py
code served (permissive licence) · get_code("bdeef284ceabe32e")

Repositories linked to this paper

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Abstract

In recent years, deep learning has become a part of our everyday life and is revolutionizing quantum chemistry as well. In this work, we show how deep learning can be used to advance the research field of photochemistry by learning all important properties for photodynamics simulations. The properties are multiple energies, forces, nonadiabatic couplings and spin-orbit couplings. The nonadiabatic couplings are learned in a phase-free manner as derivatives of a virtually constructed property by the deep learning model, which guarantees rotational covariance. Additionally, an approximation for nonadiabatic couplings is introduced, based on the potentials, their gradients and Hessians. As deep-learning method, we employ SchNet extended for multiple electronic states. In combination with the molecular dynamics program SHARC, our approach termed SchNarc is tested on a model system and two realistic polyatomic molecules and paves the way towards efficient photodynamics simulations of complex systems.

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